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All truth passes through three stages. First, it is ridiculed. Second, it is violently opposed. Third, it is accepted as being self-evident. - Arthur Schopenhauer -
It is normal for batteries in bad condition to show a high voltage then drop as the battery is being desulfated. Once the battery is desulfated enough to hold a charge you will see the voltage start to climb again. Keep in mind though that if the battery is damaged one or more of the cells may not take a charge at all.
There is lots of valuable information already posted in this forum. If you use the search tool you can find threads directly related to the self pulsing relay that you are using.
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Relay Charger Battery Conditioning Question
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